题目: | Amorphous (lysine)2PbI2 layer enhanced perovskite photovoltaics |
作者: | Yehui Wen1,2#, Tianchi Zhang1,2#, Xingtao Wang3#, Tiantian Liu4#, Yu Wang5, Rui Zhang5, Miao Kan6, Li Wan7, Weihua Ning2*, Yong Wang1* & Deren Yang1* |
摘要: | Passivation materials play a crucial role in a wide range of high-efficiency, high stability photovoltaic applications based on crystalline silicon and state-of-the-art perovskite materials. Currently, for perovskite photovoltaic, the mainstream passivation strategies routinely rely on crystalline materials. Herein, we have invented a new amorphous(lysine)2PbI2 layer-enhanced halide perovskite. By utilizing a solid phase reaction between PbI2 and lysine molecule, an amorphous (lysine)2PbI2 layer is formed at surface/grain boundaries in the perovskite films. The amorphous (lysine)2PbI2 with fewer dangling bonds can effectively neutralize surface/interface defects, achieving an impressive efficiency of 26.27% (certified 25.94%). Moreover, this amorphous layer not only reduces crystal lattice stress but also functions as a barrier against the decomposition of organic components, leading to suppressed de-structuring of perovskite and highly stable perovskite solar cells. |
影响因子: | 14.7 |
分区情况: | 一区 |